A few complexes of copper(II), nickel(II), cobalt(II), Zinc(II), tin(IV) and cadmium(II) with two newly synthesized organometallic compounds, 1Formylferrocene phenylNthiosemicarbazone (HFfptsc) and 1acetyl ferrocene phenyl Nthiosemicarbazone (HAfptsc) have been isolated. The interaction of (HFfptsc) with Me2SnCl2 and MeSnCl3. Yield a series of organotin (IV) compounds. The reactivity of MeSn(Ffptsc)2Cl towards MeSH, Me2N SiMe3, Me2NsiMe3, SiMe3N3, and Me3SiCCPh are also described. These complexes have been characterized on the basis of elemental analysis, molecular weights, molar conductances, magnetic moments and spectroscopic (IR, 1HNMR, UVvis) data.